Intense few-cycle laser pulses have a breadth of applications in high energy density science, including particle acceleration and x-ray generation. Multi-amplifier laser system pulses have durations of tens of femtoseconds or longer. To achieve high intensities at the single-cycle limit, a robust and efficient post-compression scheme is required. We demonstrate a staged compression technique using self-phase modulation in thin dielectric media, in which few-cycle pulses can be produced. The few-cycle pulse is then used to generate extreme ultravoilet light via high harmonic generation at strong field intensities and to generate MeV electron beams via laser solid interactions at relativistic intensities.

Thin-film compression (TFC) and the focusability of high-power laser pulses after self-phase modulation in thin films at transport intensities (∼1 TW∕cm 2 ) for petawatt laser systems is demonstrated. High-energy (∼296 mJ) laser pulses are compressed from ∼55 fs to ∼31 fs. Additionally, the focusability of high-power (∼45–55 TW) flat-top laser pulses after spectral broadening in thin films is found to be largely maintained, showing only modest decreases in the energy contained in the central part of the focal spot. In light of these findings, TFC offers a method for moving toward single-cycle pulse durations at significantly higher energies than those found at present, and if beam instabilities can be mitigated, maybe even higher intensities.