A Preliminary Design Study For The HYPER System: Won S. Park, Tae Y. Song, Byoung O. Lee, Chang K. Park
A Preliminary Design Study For The HYPER System: Won S. Park, Tae Y. Song, Byoung O. Lee, Chang K. Park
A Preliminary Design Study For The HYPER System: Won S. Park, Tae Y. Song, Byoung O. Lee, Chang K. Park
www.elsevier.com/locate/ned
Abstract
In order to transmute the long-lived radioactive nuclides such as transuranics (TRU), Tc-99, and I-129 in LWR spent
fuel, a preliminary conceptual design study has been performed for an accelerator driven subcritical reactor system,
called HYPER (HYbrid Power Extraction Reactor). The core has a hybrid neutron energy spectrum which includes fast
and thermal neutrons for the transmutation of TRU and fission products, respectively. TRU are loaded into the
HYPER core in a TRU /Zr metal form because a metal type fuel has very good compatibility with the pyro-chemical
process which retains the self-protection of transuranics at all times. On the other hand, Tc-99 and I-129 are loaded as
pure technetium metal and sodium iodide, respectively. Pb /Bi is chosen as a primary coolant because Pb /Bi can
provide a good spallation target and produce a very hard neutron energy spectrum. As results, the HYPER system does
not need any independent spallation target system. 9Cr /2WVTa is used as a window material because this advanced
ferritic/martensitic steel is known to have a good performance in the highly corrosive and radiative environment. The
support ratios of the HYPER system are about 4 /5 for TRU, Tc-99, and I-129. Therefore, a radiologically clean
nuclear power, i.e. zero net production of TRU, Tc-99 and I-129 can be achieved by combining 4 /5 LWRs with one
HYPER system. In addition, the HYPER system, having good proliferation resistance and high nuclear waste
transmutation capability, is believed to provide a breakthrough to the spent fuel problems the nuclear industry is facing
with.
# 2002 Elsevier Science B.V. All rights reserved.
1. Introduction
Nuclear is being emerged as one of the most
promising sustainable energy sources for the 21st
century. Many evolutionary or innovative concepts are being investigated as a future nuclear
system. Not a single system is supposed to meet
the requirement, radiological cleanliness the future nuclear system has to satisfy. The combina-
Corresponding author
E-mail address: [email protected] (W.S. Park).
0029-5493/02/$ - see front matter # 2002 Elsevier Science B.V. All rights reserved.
PII: S 0 0 2 9 - 5 4 9 3 ( 0 2 ) 0 0 2 0 7 - 8
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W.S. Park et al. / Nuclear Engineering and Design 219 (2002) 207 /223
2. Core concept
The basic requirements for the core design are to
maximize the proton beam current efficiency, the
W.S. Park et al. / Nuclear Engineering and Design 219 (2002) 207 /223
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210
W.S. Park et al. / Nuclear Engineering and Design 219 (2002) 207 /223
Table 1
Design parameters of the core
Parameters [unit]
Values
System
Core thermal power [MW]
Core inlet/outlet temperature (8C)
Active core height [m]
Effective core diameter [m]
System multiplication factor
Accelerator beam power [MW]
Average discharge burnup [%at.]
TRU transmutation capability [kg per year]
Number of fuel assemblies
Average linear power density [kW m 1]
No. of burnable absorber rods per assembly
1000
340/510
1.6
2.6
0.98
/10 /20
/25
258
225
12.48
7
Assembly
Assembly pitch (cm)
Pitch-to-diameter
Tube thickness (cm)
Tube material
Rods per assembly
16.13
1.48
0.3556
HT-9
217
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Table 2
External neutron source multiplication for various core configurations
Case no.
Multiplicitya
Power peaking
Core configuration
1
2
3
4
5
39.4
35.7
25.8
16.9
31.4
12.05
13.51
17.55
25.71
14.22
1.859
1.273
1.223
1.327
1.289
Uniform loading
3 Zones without FP Ass.
3 Zones with FP Assemblies in the middle core
3 Zones with FP Assemblies in the inner core
3 Zones with FP Assemblies in the outer core
a
b
W.S. Park et al. / Nuclear Engineering and Design 219 (2002) 207 /223
Table 3
Variation of actinide concentration at the 20th cycle
Nuclide
Inventory (kg)
U-233
U-234
U-235
U-236
U-238
Np-237
Pu-238
Pu-239
Pu-240
Pu-241
Pu-242
Am-241
Am-242
Am-242m
Am-243
Cm-242
Cm-243
Cm-244
Cm-245
Cm-246
BOC
EOC
Variation
0.2144E/02
0.9166E/01
0.3203E/01
0.3949E/01
0.9675E/03
0.7585E/02
0.1456E/03
0.8774E/03
0.1299E/04
0.2797E/03
0.3898E/03
0.1049E/03
0.7905E/01
0.9818E/01
0.1191E/03
0.8502E/01
0.1090E/01
0.1142E/03
0.3564E/02
0.3084E/02
0.1902E/02
0.9215E/01
0.3121E/01
0.3986E/01
0.9516E/03
0.6977E/02
0.1432E/03
0.8082E/03
0.1270E/04
0.2674E/03
0.3845E/03
0.1010E/03
0.7898E/01
0.9773E/01
0.1182E/03
0.8498E/01
0.1081E/01
0.1142E/03
0.3571E/02
0.3072E/02
/0.0002
/0.039
/0.082
/0.037
/15.9
/6.08
/2.40
/69.2
/29.0
/12.3
/5.3
/3.9
/0.0001
/0.045
/0.9
/0.004
/0.009
0.0
/0.07
/0.12
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W.S. Park et al. / Nuclear Engineering and Design 219 (2002) 207 /223
214
Table 4
Design specifications of fuel rod
Parameters
Fuel type
Alloy fuel
Dispersion fuel
Fuel slug
4.58
50 wt.% TRU-50 wt.% Zr
12.36
6.18
5.18
45 wt.% (TRU /10 Zr) /55 wt.% Zr
9.16 (TRU /10Zr: 18.37)
3.7
Cladding (mm)
5.28
6.70
0.71
5.28
6.70
0.71
12.48
12.48
Inside dia
Outside dia
Thickness
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216
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Fig. 11. Rod deformation rate for the dispersion and alloy type.
W.S. Park et al. / Nuclear Engineering and Design 219 (2002) 207 /223
217
for casting the Technetium metal has been developed and irradiation experiments did not show
any evidence of the swelling or disintegration of
the metal (OECD/NEA, 1998). On the other hand,
an elemental form is found to be unacceptable for
Iodine because of its volatility and chemical
reactivity. Thus, metal iodides are being considered. Sodium iodide (NaI) and calcium iodide
(CaI2) are the desirable forms. Sodium iodide is
expected to have melting problems when the
sodium is liberated from iodide due to the
transmutation.
3.4. Fission product target design configuration
(Park et al., 2000)
Thermal neutrons are much more efficient for
the transmutation of Tc-99 and I-129 than fast
ones. The evaluation shows that the transmutation
rate can be improved considerably then. In order
to have a thermal neutron spectrum in the
HYPER system, some moderation has to be
included. Graphite and calcium hydride have
been studied in terms of their effectiveness for
moderation. The comparative study shows that a
calcium hydride is much better for the production
of localized thermal neutrons.
The introduction of a moderator causes power
peaking problems in the TRU assemblies that
surround the FP target. Many types of target
configurations were investigated in terms of power
peaking and transmutation rate. The configuration where Tc-99 is loaded as a plate type in the
outer-most region and I-129 is loaded as NaI rods
mixed with CaH2 rods in the inner region was
concluded to be the best. Fig. 12 shows the
configuration of FP target. Monte Carlo transport
code, MCNAP has been used with ENDF/B-VI
data library for the design of fission product target
as it is in the core design. Fission product target
and the TRU assemblies surrounding fission
product target were described by pin-by-pin
model. The designed FP target configuration is
estimated to have the transmutation capability of
57.8 and 13 kg per year for Tc-99 and I-129,
respectively when 6 FP targets are loaded. The
support ratios of the HYPER system for Tc-99
and I-129 are estimated to be 5.7 and 4.0,
respectively. The support ratio for Tc-99 is much
larger while that for I-129 is slightly less compared
with the support ratio for TRU.
Fig. 13 shows the neutron energy spectra in the
region of fission product target. The spectrum in
the fuel assemblies surrounding the FP target is
relatively softer than that of normal fuel assemblies. This softened spectrum causes an increment
to the local power. The calculation predicted a
local power peak of 1.232, which is within the
acceptable range. In addition, the loading of FP
targets makes the core coolant void coefficients
more negative, but the Doppler coefficient less
negative. It can be concluded that the FP target
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4. Cooling system
4.1. Basic configuration
A Lead /Bismuth (Pb /Bi) eutectic alloy was
selected as a coolant material for the HYPER
system. The advantages expected from Pb /Bi
cooling are:
1) Pb /Bi has good nuclear properties, i.e. low
absorption cross-sections and low moderating
power, which is quite desirable for the incineration of TRU.
2) Pb /Bi can be used as an excellent spallation
target itself. Using Pb /Bi as a coolant removes the necessity of an independent target
and its cooling system.
3) Pb /Bi has good cooling capabilities and heat
transfer characteristics, i.e. high boiling temperature and high heat transfer rate.
4) Pb /Bi coolant system has enhanced safety
characteristics. It has no violent reaction with
air or water and it is an effective gamma
shielding material.
On the other hand, some problems have to be
solved for the use of Pb /Bi as a coolant. Pb /Bi is
highly corrosive to structural materials. The corrosion problems are major issues, which limit wide
use of Pb /Bi as a coolant material. In addition,
Pb /Bi requires higher pumping power than alkali
metals or water to operate a cooling system
because of its higher density.
The thermal efficiency of the power cycle
strongly depends on the temperature at which
heat is supplied by the primary to the secondary
coolant. It is obvious that the coolant temperature
should be set as high as possible for an optimum.
However, mechanical and corrosion characteristics of structural materials set the upper limit.
According to Russian results (Adamov et al., 1997;
Yachmenyov et al., 1998), the maximum allowable
temperature of Pb /Bi coolant is approximately
650 8C. The lower limit of the coolant tempera-
W.S. Park et al. / Nuclear Engineering and Design 219 (2002) 207 /223
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W.S. Park et al. / Nuclear Engineering and Design 219 (2002) 207 /223
Table 5
Results of the sub-channel analysis
Parameter
510.0
612.0
524.2
634.8
536.7
654.7
32.6
32.8
Inlet velocity (m s 1 )
Average
Interior
Edge
Corner
Inter gap
1.433
1.449
1.382
1.097
0.000
1.433
1.449
1.382
1.097
0.000
W.S. Park et al. / Nuclear Engineering and Design 219 (2002) 207 /223
221
effectiveness of beam and to minimize the radiation damage and mechanical stress of the beam
window (Song et al., 2000).
5.2. Performance analysis
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W.S. Park et al. / Nuclear Engineering and Design 219 (2002) 207 /223
Table 6
Characteristics of the target design
Parameter
Beam window
Material
Structure
Diameter/thickness
(cm)
Characteristics
9Cr /2WVTa
Cylinder with circular shape end (single
window)
40/0.2
Beam
Incoming beam
mutually exclusive requirements. The core geometry is designed based on the spallation neutron
efficiency rather than the negative void coefficient
concern. The uranium recovery rate from LWR
spent fuel is assumed to be 99.9% for the core
analysis. The uranium fraction becomes about 20
wt.% of heavy metal when the core nuclide
composition reaches at a pseudo equilibrium
status. In order to reduce the reactivity swing
due to the lack of fertile nuclides, a burnable
absorber is considered. Either alloy or dispersion
type metallic fuels are being considered for the
HYPER system. A dispersion type fuel is supposed
to give better irradiation performance compare to
an alloy type fuel. Pb /Bi is used as a coolant and a
loop concept is preferred as a primary cooling
system. The basic analysis shows that three loops
are optimal to the HYPER system. Each loop has
one super heater and two evaporators. A single
window with a thickness of 2 mm 9Cr /2WVTa is
designed to provide the HYPER core with 1 GeV,
10/20 mA protons. The HYPER system is expected to transmute about 258 kg of TRU, 57.8 kg
of Tc-99 and 13 kg of I-129 and produce 1000
MWth through the transmutation process. The
support ratios of the HYPER system are about 4 /
5 for TRU, Tc-99, and I-129. Therefore, a radiologically clean nuclear power, i.e. with zero net
production of TRU, Tc-99 and I-129 can be
achieved by combining 4/5 LWRs with one
HYPER system.
The developed concept is supposed to have
some uncertainties because there are not much
experimental data available on TRU /Zr fuel and
Pb /Bi coolant/target. Some experiments are
scheduled to verify those fuel and coolant/target
design concepts during 2001/2003.
6. Summary
The design goal of the HYPER system is to
transmute TRU, Tc-99, and I-129. Major consideration has been given to the maximization of the
transmutation capability. A fast neutron spectrum
is more preferable for the transmutation of TRU
while a thermal neutron spectrum is better for Tc99 and I-129. The HYPER core is designed to have
hybrid neutron spectra in order to meet both
Acknowledgements
The authors give many thanks to Dr Yong H.
Kim and Nam I. Tak for their invaluable contributions. The authors also appreciate the financial support of MOST (Minister of Science and
Technology) for the HYPER system development.
W.S. Park et al. / Nuclear Engineering and Design 219 (2002) 207 /223
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