PhysRevLett.124.210605
PhysRevLett.124.210605
PhysRevLett.124.210605
We report a systematic study of finite-temperature spin transport in quantum and classical one-
dimensional magnets with isotropic spin interactions, including both integrable and nonintegrable models.
Employing a phenomenological framework based on a generalized Burgers’ equation in a time-dependent
stochastic environment, we identify four different universality classes of spin fluctuations. These comprise,
aside from normal spin diffusion, three types of superdiffusive transport: the Kardar-Parisi-Zhang
universality class and two distinct types of anomalous diffusion with multiplicative logarithmic corrections.
Our predictions are supported by extensive numerical simulations on various examples of quantum and
classical chains. Contrary to common belief, we demonstrate that even nonintegrable spin chains can
display a diverging spin diffusion constant at finite temperatures.
DOI: 10.1103/PhysRevLett.124.210605
Introduction.—Obtaining a theoretical framework that is comprising both the Drude weights [27–30] and diffusion
able to explain how macroscopic laws of transport emerge constants [20,31–34], together with a myriad of other
from the microscopic deterministic dynamics presents one applications [35–41]. This provided a coherent picture
of the central challenges of condensed matter physics. This for earlier numerical results (see, e.g., Refs. [42–46] and
transcends purely academic interest, as many problems of references therein). Despite these developments, the dis-
quantum transport remain unresolved in the presence of covery of superdiffusive spin transport and KPZ scaling
strong interactions [1,2]. One viable strategy to improve our [cf. Eq. (4)] in integrable spin chains with isotropic
understanding of transport phenomena is to identify uni- interactions, originally discovered numerically in the
versality classes and study certain representative instances Heisenberg spin-1=2 chain in Refs. [47,48] and further
which can either be solved exactly, or at least simulated surveyed in Refs. [49–53], came as a surprise. Although
numerically in an efficient manner [3–6]. In this respect, recent numerical works [52,54–56], in combination with
interacting many-particle systems confined to one spatial scaling arguments explaining the dynamical exponent [50],
dimension, in the realms of both quantum and classical constitute convincing evidence in support of the KPZ
models, take a special role as they often exhibit anomalous universality, a rigorous analytical account of this phenome-
features [7,8]. One of the prominent examples of a non- non is still lacking. Most recent studies suggest that
equilibrium universality class is given by the Kardar-Parisi- anomalous spin transport occurs only in integrable systems
Zhang (KPZ) equation [9], which is widespread in the area invariant under non-Abelian [SU(2) or SO(3)] Lie groups.
of growing one-dimensional interfaces [10,11]. The KPZ In contrast, normal spin diffusion is expected to be immedi-
and Lévy universality classes, which also occur in systems ately recovered upon breaking integrability [52,56]. The
of classical particles, can be understood in the scope of the occurrence of normal diffusion in nonintegrable symmetric
nonlinear fluctuating hydrodynamics [12–16]. chains was also suggested in the numerical study [57] (see
In recent years, the advent of the generalized hydro- also Refs. [53,56]) after a long-lasting controversy [58–63].
dynamics [17,18], studies of quantum chaos and its relation With the aim to resolve these controversies and giving
to transport [19–23], and of noisy quantum systems a comprehensive description of spin transport in these
[24–26], reinvigorated the field of transport laws in spin systems, in this Letter we address two key open questions:
chain models. In integrable quantum chains, a closed-form (i) Do nonintegrable homogeneous spin chains always
universal expression for the conductivity matrix was found, display normal diffusive spin transport? (ii) What are all
possible types of spin transport exhibited by rotationally and classical spin systems with isotropic interactions
invariant chains? valid on large spatiotemporal scales. Here we propose an
To address these questions, we carry out a systematic effective description, which is inherently classical in nature,
study of magnetization transport in classical and quantum by employing the continuum theory for a classical spin
spin systems in the nonmagnetized sector of thermal field, which is in turn treated within a hydrodynamic
equilibrium states where the global rotational symmetry approximation. Microscopic details are included implicitly
remains unbroken. Aiming at complete classification of through an appropriate phenomenological noise.
admissible transport laws, we build on a recent work by As our starting point, we consider the most general
Bulchandani [53] and devise a simple phenomenological form of a manifestly SO(3)-symmetric Hamiltonian equa-
model that helps us to single out two novel nonequilibrium tion of motion,
universality classes of spin transport. We corroborate our
δH
findings with extensive numerical simulations of classical S⃗ t ¼ −S⃗ × ⃗ S⃗ x ; S⃗ xx ; …;
¼ F ½S; ⃗ ¼ 1;
jSj ð1Þ
and quantum chains. Quite unexpectedly, we find that the δS⃗
answer to question (i) is negative: Surprisingly, the spin
diffusion constant is found to diverge logarithmically in time specified by some functional F involving scalar and vector
in rotationally invariant nonintegrable chains, thus refuting a products of the spin field and derivatives thereof. We can
widely held belief that nonintegrable models cannot display include classical lattice models as well, which are analyzed
infinite diffusion constants at finite temperatures. through their continuum counterparts. To additionally
Moreover, we find that rotationally invariant integrable incorporate quantum spin chains, we first perform a
chains can display different universal transport dynamics, mean-field average [64] of the microscopic spin
from KPZ-type to normal diffusive. Hamiltonian. It has to be stressed that such a correspon-
Therefore, from our perspective the results summarized dence cannot retain all quantitative features of spin
in Fig. 1 provide a comprehensive classification of dynamics. Nonetheless, we shall argue, in the spirit of
magnetization transport in homogeneous rotationally Ref. [53], that correspondence is still meaningful to capture
invariant quantum and classical spin models, nonintegrable the correct large-time transport behavior.
and integrable, and give a comprehensive response to The outlined effective theory applies in thermal equi-
question (ii). librium in the nonmagnetized sector (i.e., at half-filling)
We proceed by first introducing the formalism of an where the global rotational invariance of the underlying
effective spin field theory which we relate to the KPZ invariant measure is unbroken. This is of paramount
equation in a time-dependent noisy environment. To importance for the anomalous character of magnetization
systematically test our predictions, we subsequently con- dynamics, as the addition of finite chemical potential
centrate on a number of simple representative examples. (or external magnetic field), which dynamically breaks
Spin-field theory of isotropic magnets.—In order to the non-Abelian symmetry, leads to restoration of normal
capture various universality classes of spin superdiffusion, spin diffusion (accompanied in integrable systems by a
the task at hand is to devise an effective theory for finite spin Drude weight [66] or ballistic current). On large
finite-temperature magnetization dynamics in quantum spatiotemporal scales, the evolution of a spin field is
accurately captured by a “hydrodynamic soft mode”
carrying a negligible energy density, which can be con-
veniently described in terms of two intrinsic geometric
quantities, curvature κ ¼ ðS⃗ x · S⃗ x Þ1=2 and torsion τ ¼ κ −2 S⃗ ·
ðS⃗ x × S⃗ xx Þ. The soft mode pertains to the long-wavelength
[k ∼ Oð1=lÞ] limit of the spin procession (about a dis-
tinguished axis fixed by the perturbation which breaks the
gauge invariance assumed subsequently to be the z axis)
at constant
pffiffiffiffiffiffiffiffiffiffiffiffi ffi latitude Sz ¼ h, with Sx ðx; tÞ iSy ðx; tÞ ¼
1 − h exp ½iðkx þ wtÞ, frequency wðkÞ ¼ −k2 h, and
2
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nonintegrable systems [33,68]), they can be effectively For n ¼ 2, Eq. (2) is just the ordinary noisy Burgers’
decoupled from the fluctuations of the torsion field pro- equation equivalent to the KPZ equation, up to a change of
vided the latter are superdiffusive. Based on this, we can variable [9]. A recent work [69] examined the properties of
conclude that torsion τ remains the only relevant scalar such KPZ equations with time-dependent noise term
field at large times and that, since τ ∼ h at small h, the of the form (3), finding nonuniversal large-time behavior
⃗
finite-temperature spin-spin fluctuations hSðx; ⃗
tÞ · Sð0; 0Þi for ζ > 1=2 and universal KPZ dynamics (with modified
are proportional to fluctuations of the torsional mode dynamical exponents) for ζ ≤ 1=2. Exactly at the “critical”
hτðx; tÞτð0; 0Þi. We shall assume that such a decoupling point ζ ¼ 1=2 corresponding precisely to diffusive spread-
mechanism holds generically for equations of the form (1). ing of microscopic excitations, in Ref. [69] the authors
Generalized noisy Burgers’s equation.—To account for deduce a modified diffusive scaling x ∼ t1=2 log2=3 ðt=t0 Þ
thermal fluctuations, we invoke the standard arguments (for the particular case the scaling should be understood
of the nonlinear fluctuating hydrodynamics (NLFHD) [14], as a lower bound and not a rigorous statement [70], as
where the microscopic degrees of freedom of the under- numerics are not able to distinguish slightly different
lying Hamiltonian dynamics are effectively taken into exponents; see also additional numerical data in Ref. [71]).
account through an appropriate stochastic term and effec- Keeping this in mind, the statistics of spin fluctuations in
tive diffusion (i.e., dissipation). This brings us to the this case is expected to exhibit a crossover from an effective
generalized noisy Burgers’ equation of the form KPZ dynamics at short-intermediate times t ≃ t0 ,
pffiffiffi
τt þ ðτn þ Dτx þ γ ηÞx ¼ 0; ð2Þ ⃗
hSðx; ⃗
tÞ · Sð0; 0Þi ≃ t−2=3 f KPZ ðΓKPZ xt−2=3 Þ; ð4Þ
where D ¼ γ=χ τ is the phenomenological diffusion con- to the asymptotic scaling of the form
stant, χ τ is static susceptibility of τ, ηðx; tÞ a white noise
with unit variance, γ is the effective variance of the noisy G½ΓG xt−1=2 log−2=3 ðt=t0 Þ
environment, and parameter n ≥ 2 specifies the degree of ⃗
hSðx; ⃗
tÞ · Sð0; 0Þi ≃ ; ð5Þ
t1=2 log2=3 ðt=t0 Þ
nonlinearity. From the general scaling relations τðx; tÞ ≃
t−1=2z fðxt−1=z Þ and hτðx; tÞτð0; 0Þi ≃ t−1=z gðxt−1=z Þ (here 2
and below, the bracket refers to the average with respect with Gaussian profile GðxÞ ≃ e−x in the limit t ≫ t0 .
to the canonical invariant measure), one however deduces The anomalous form (5) implies a divergent behavior
that z ¼ ðn þ 1Þ=2, which implies that nonlinearities of DðtÞ ∼ ½logðtÞ4=3 .
degree n ≥ 4 (with z > 2) are subdiffusive and thus Integrable isotropic magnets.—Our main example is the
R
irrelevant at large times. Although NLFHD has no pre- Heisenberg continuous magnet Hð2Þ ¼ 12 dxS⃗ x · S⃗ x (using
dictive power in this case, one generically expects to find standard notation S⃗ x ¼ ∂ x S,
⃗ etc., for partial derivatives),
normal spin transport. also known as the isotropic Landau-Lifshitz model [75,76],
The final key ingredient is to impose the structure of the which is a paradigmatic example of an integrable classical
noise, reflecting the nature of fluctuating modes which are field theory. The time evolution is governed by the non-
relevant on a hydrodynamic scale. In the spirit of conven- ð2Þ
tional NLFHD (see, e.g., Ref. [14] for application to linear partial differential equation S⃗ t ¼ FLL ¼ S⃗ × S⃗ xx .
This equation possesses an infinite family of
anharmonic chains), in the presence of long-lived ballis- R
tically propagating normal modes of Euler hydrodynamics, Hamiltonians HðnÞ in involution, e.g., H ð3Þ ¼ 12 dxS⃗ ·
R
we adopt a time-independent white noise γ ¼ γ 0 . The same ðS⃗ x × S⃗ xx Þ and Hð4Þ ¼ − 12 dx½S⃗ xx · S⃗ xx − 54 ðS⃗ x · S⃗ x Þ2 .
applies to integrable systems which exhibit extensively Invoking the “decoupling hypothesis” and the phenom-
many local conserved fields, as previously suggested in enological noisy environment, the torsional mode in each
Ref. [53]. On the contrary, generic spin systems do not HðnÞ is governed by the generalized Burgers’ equations (2)
support ballistic modes and excitations dissipate through with nonlinearity of degree n (see also Ref. [71] for the
the system. In this case, the variance γ is expected to obey details). Adopting a constant value for γ, the dynamics falls
the diffusive scaling and decay with time into the KPZ class at the lowest order n ¼ 2. This is,
however, no longer the case for n > 2 where the quadratic
γ ≡ γðtÞ ∼ ½t0 =ðt0 þ tÞζ with ζ ¼ 1=2; ð3Þ nonlinearity is absent. For n ≥ 4, the nonlinearity is
dominated by diffusive processes, and Hamiltonians
where t0 denotes an unknown model- and temperature- Hðn>3Þ thus do not display any enhancement of normal
dependent scale. The picture behind this is that fluctuations diffusion. The cubic n ¼ 3 case is however marginally
excited by the spatiotemporal variation of the chemical irrelevant in the dynamic renormalisation group sense. This
potential should dissipate away diffusively as their density type of nonlinearity has been previously examined in the
decays to zero with exponent ζ ¼ 1=2. study of Toom interface [77–79] and argued to result in a
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PHYSICAL REVIEW LETTERS 124, 210605 (2020)
spin-S chains [52] concluded in favor of normal spin Finally, It is reasonable to expect that the divergence (6)
diffusion (z ¼ 2) in nonintegrable spin chains (S ≥ 1). could be seen in a real experimental setting, and we hope
Here we prefer to facilitate a direct comparison with that this can be successfully addressed in the near future.
classical spin chains. To this end, we carried out time
We thank G. Barraquand, B. Bertini, V. Bulchandani,
dependent matrix renormalization group simulations
P. Le Doussal, Ž. Krajnik, J. Moore, T. Prosen, and H.
[83–85] of the quantum anisotropic spin-1 chain Ĥ δ and, Spohn for extensive and illuminating discussions, and the
restricting ourselves to only moderately small δ, numeri- organizers of the workshop “Thermalization, Many-Body-
cally extracted the spin diffusion constant from the time- Localization and Generalized Hydrodynamics” at the ICTS
dependent dc conductivity with a diffusive tail σðtÞ ≃ Bangalore for hospitality, where parts of this work were
ðχ=TÞD þ ct−1=2 with spin susceptibility χ and fitting carried out. J. D. N. is supported by the Research
parameters D and c; see additional numerical data in Foundation Flanders (FWO). E. I. is supported by the
Ref. [71]. The data shown in Fig. 2 indicate that the spin Slovenian Research Agency under the Programme
dynamics in the nonintegrable spin-1 chain mirrors that of P1-0402 and NWO Talent Programme Veni Grant
its classical counterparts and thus experiences the same No. 680-47-454 by the Netherlands Organisation for
ð2Þ
divergence (6) (Dlog class). Notice that in the quantum Scientific Research. C. K. acknowledges support by the
integrable S ¼ 1=2 chain, the divergence in the δ → 0þ Deutsche Forschungsgemeinschaft through the Emmy
limit is different as it diverges polynomially as D ∼ δ−1=2 Noether program (Grant No. KA 3360/2-1).
[20,32], signaling the onset of the KPZ dynamical exponent
at δ ¼ 0.
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