Kasmudin 2022 J. Phys. Conf. Ser. 2377 012048
Kasmudin 2022 J. Phys. Conf. Ser. 2377 012048
Kasmudin 2022 J. Phys. Conf. Ser. 2377 012048
Series
*Email: [email protected]
Abstract. The e-beam produced by the high-energy electron accelerator has a relatively small
penetrating power. To increase the penetrating power, a converter must convert the e-beam
energy into bremsstrahlung x-rays. This research aims to determine the optimum thickness of
tantalum, tungsten, and lead as a converter of e-beam energy into bremsstrahlung x-rays at a 10
MeV high-energy electron accelerator. The optimum thickness of tantalum, tungsten, and lead
is determined using simulation with MCNPX software. The electron source modeling with an
energy of 10 MeV is made in the form of a flat plane with a size of 120 cm by 10 cm at a distance
of 1 mm from the converter. The converter has dimensions of 160 cm by 24 cm and its thickness
varies from 1 - 7.5 mm. Then two planar detectors are placed at a distance of 2 cm in front and
behind the converter. The simulation results show that the optimum thickness for tantalum,
tungsten, and lead converter is 2.0 mm, 1.8 mm, and 2.8 mm respectively. The maximum forward
scattered bremsstrahlung x-rays energy are 2.1137 MeV, 2.1287 MeV, and 2.1850 MeV,
respectively. And the maximum conversion efficiency is 21.137%, 21.287%, and 21.850%,
respectively. These results can be used as a reference in the design of the converter for the 10
MeV high-energy electron accelerator.
1. Introduction
An electron accelerator is a device to accelerate an electron beam (e-beam) that can be used to irradiate
products according to their needs, for example, for the sterilization of various food products, agricultural
products, wires, medicines, and medical devices [1,2]. To irradiate medical device products (medical
sterilization) a high-energy e-beam of up to 10 MeV is required [3]. However, the penetrating power of
e-beam irradiation produced by electron accelerators is relatively much lower than the penetrating power
of gamma-ray irradiation produced by gamma irradiators with Co-60 sources. Therefore, for the purpose
of irradiating medical device products using high-energy electron accelerators, the energy of the e-beam
must first be converted into a bremsstrahlung x-ray (BXR) beam whose penetrating power is much
greater than that of the e-beam, it can even exceed the gamma-ray penetrating power of Co-60. E-beams
and high-energy x-ray photons are usually generated by linear accelerators [4,5].
In general, the electron accelerator parts consist of an electron source that produces an e-beam, an
accelerator tube and an e-beam accelerator system that accelerates the e-beam so that it has a certain
desired kinetic energy according to its intended use, a focusing system that functions to focusing the e-
beam so that it does not spread and does not hit the walls of the accelerator tube, a scanning window
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Published under licence by IOP Publishing Ltd 1
The 11th National Physics Seminar (SNF 2022) IOP Publishing
Journal of Physics: Conference Series 2377 (2022) 012048 doi:10.1088/1742-6596/2377/1/012048
system that functions to direct the e-beam that comes out of the electron accelerator to irradiate the
product directly using the e-beam, and a BXR converter that functions to convert the energy of the e-
beam into a continuous BXR [6] to irradiate products that require high penetrating power. In addition,
it is also necessary to have a vacuum system to vacuum the e-beam accelerator tube to 10-7 torr so that
the electrons can be accelerated without being blocked or hitting air particles in the accelerator tube.
Then there is also a need for a cooling system to cool the walls of the accelerator tube, a scanning
window system, and a BXR converter while the electron accelerator is operating. There are several
requirements to be considered in the selection and determination of the BXR converter material from e-
beam energy: thin, strong and resistant to electron collision, resistant to corrosion, high melting point,
high conversion efficiency, and if a photonuclear reaction occurs, it produces neutron particles with low
energy [7,8].
This research aims to determine the optimum thickness of tantalum, tungsten, and lead as a BXR
converter at a 10 MeV high-energy electron. If the thickness is too thin, the conversion efficiency will
be relatively low because the electron deceleration process by the atomic nucleus of the converter
material is not yet maximized. Meanwhile, if the thickness is too thick, the conversion efficiency will
also be relatively low because the converter material itself absorbs the BXR energy. So, in this research,
we will look for the optimum thickness of BXR converter material made of tantalum, tungsten, and lead
with the highest BXR conversion efficiency.
Determination of the optimum thickness of the BXR converter material as mentioned above was
carried out by simulation using the Monte Carlo N-Particle X version 2.7.0 (MCNPX v.2.7.0) software.
MCNP is computer software written using the Fortran programming language based on the Monte Carlo
method and can be used for neutron, photon, electron, or coupled neutron/photon/electron
transport [9,10]. The code of MCNP was developed at Los Alamos National Laboratory (LANL), USA
[11]. This simulation software is very well used for dosimetry analysis.
2. Method
Determination of the optimum thickness of tantalum, wolfram (tungsten), and lead as an energy
converter of e-beam to BXR on a 10 MeV high-energy electron accelerator was carried out by simulation
using MCNPX v.2.7.0 software. In general, three steps must be done, namely creating an input file,
running the input file, and interpreting the results of running (output). The first step, creating an MCNP
input file, is filling in a “card”, consisting of three cards: cell cards, surface cards, and data cards [12].
Cell cards and surface cards are geometric inputs of the object to be simulated, while data cards are
information about the material of the simulated object, the definition of radiation sources, and the
physical quantities to be calculated (tally). After creating the MCNP input file, the second step is to run
the input file with the MCNP code using an Intel (R) Core (TM) i7-8750H CPU @ 2.20 GHz 2.21 GHz,
8.00 GB RAM. After running the input file with the MCNP code, the third step is to take the data from
the MCNP code output, which is needed for further interpretation and analysis. One of the most
important things in the simulation is that the geometry modeling is made according to the real condition
in terms of shape, size, and composition of the elements that make up the BXR converter. Then the
definition of a radiation source includes the form of the source, the type of radiation emitted, the energy
of each particle, the position of the source, and the direction of the emitted particle beam [10].
The simulation steps for determining the optimum thickness of tantalum, tungsten, and lead as a BXR
converter are started by creating an input file for each x-ray converter material with dimensions of 160
cm high by 24 cm wide and varying thickness. The thicknesses are 1.0, 1.2, 1.4, 1.6, 1.8, 2.0, 2.2, 2.4,
2.6, 2.8, 3.0, 3.2, 3.4, 3.6, 3.8, 4.0, 4.5, 5.0, 6.0, and 7.5 mm. An e-beam source with an energy of 10
MeV is in the form of a rectangular field measuring 120 cm high by 10 cm wide with a distance of 1
mm from the surface of the x-ray converter. Then two surface detectors each measuring 300 cm by 300
cm were installed at a distance of 2 cm in front and behind the x-ray converter. The simulation
environment is created in a vacuum chamber. The tally F2 is used to calculate the flux of x-ray photons
that penetrate the detector surface in front and behind the converter. BBREM is used to reduce the
calculation uncertainty of higher BXR energy generated by the x-ray converter. The BXR produced by
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The 11th National Physics Seminar (SNF 2022) IOP Publishing
Journal of Physics: Conference Series 2377 (2022) 012048 doi:10.1088/1742-6596/2377/1/012048
the converter is emitted in all directions. In practice, the x-rays to be used are x-rays emitted in the
direction of the e-beam motion from the source to irradiate the product (in the forward direction).
Therefore, the determination of the optimum thickness of the BXR converter material is calculated based
on the energy conversion efficiency of 10 MeV electrons into BXR, which is emitted in the forward
direction. In this study, each simulation was carried out with nps (number of particle simulations) of
100000 (one hundred thousand).
The MCNP output result is the average value of the simulation of one particle or one photon. So, the
BXR energy produced by the x-ray converter is the average BXR energy converted from each electron
with a kinetic energy of 10 MeV and emitted randomly in all directions. Therefore, to get the average
energy of BXR emitted in the forward direction, it must be multiplied by the fraction of the number of
x-ray photons emitted in the forward direction to the total number of x-ray photons emitted forward and
backward. To calculate the number of x-ray photons emitted forward and backward by the x-ray
converter material, tally F2 and multiplication factor (FMn) are used according to the e-beam current
used. This study uses an electron accelerator with an electron kinetic energy of 10 MeV and an
accelerator power of 50 kW, so that the number of electrons produced by the accelerator or FMn used
in this simulation can be calculated, which is 3.12109863E+16 particle/s
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The 11th National Physics Seminar (SNF 2022) IOP Publishing
Journal of Physics: Conference Series 2377 (2022) 012048 doi:10.1088/1742-6596/2377/1/012048
the converter material [14]. So, the self-absorption of the converter material plays a role in keeping the
amount of BXR energy produced from increasing significantly after reaching a certain thickness.
For the converter materials made of tantalum up to a thickness of 2.8 mm, the ability to convert
electron energy into BXR energy increases significantly, and after passing through a thickness of 2.8
mm the conversion ability decreases and is relatively stable. The same applies to x-ray converters made
of tungsten and lead at thicknesses of 2.6 mm and 3.6 mm, respectively. Here, it appears that there is a
relation between the thickness of the x-ray converter material where the conversion ability decreases
and is relatively stable inversely proportional to the density of the converter material (converter
thickness limit: Pb 3.6 mm > Ta 2.8 mm > W 2.6 mm, while Pb < Ta < W).
4.0 90
85
3.0 75 W
70
2.5 Pb
65
60
2.0
Ta 55
1.5 W 50
Pb 45
1.0 40
0.5 35
30
0.0 25
0.0 1.0 2.0 3.0 4.0 5.0 6.0 7.0 8.0 0.0 1.0 2.0 3.0 4.0 5.0 6.0 7.0 8.0
X-Ray Converter Thickness (mm) X-Ray Converter Thickness (mm)
Figure 1. The relationship of the BXR average Figure 2. The relationship of the forward scattered
energy to the x-ray converter thickness. BXR beam fraction to the converter thickness.
Figure 2 shows the relation of the forward scattering BXR beam fraction (expressed in %) to the x-
ray converter thickness (in mm) for tantalum, tungsten, and lead materials. In general, the three x-ray
converter materials show the same characteristics. The thicker the x-ray converter material, the smaller
the forward scattering BXR beam fraction, because the converter material itself absorbs more x-ray
photon beams. Figure 2 also shows that at the same thickness of the converter material, the greater the
density of the converter material, the smaller the fraction of the BXR beam that is scattered forward. It
can be explained that the greater the density of the converter material, the greater the number of atoms
per unit volume. This results in more interactions and physical processes occurring between the incident
electrons and the resulting BXR photons.
In practice, in the use of a 10 MeV high-energy electron accelerator with e-beam energy converted
into BXR photon beam energy using an x-ray converter, not all of the x-ray photon energy beams
produced can be utilized because in fact the BXR photon beam is scattered randomly to all directions.
Meanwhile, the target of the irradiation product can only receive a beam of BXR photons that are
scattered forward.
Therefore, this research is important to calculate the average energy of BXR photons that are
scattered forward to irradiate the irradiation product as needed. To calculate the average energy of the
BXR photons emitted forward, it is necessary to first calculate the fraction of the x-ray photon beam
emitted forward as shown in Figure 2 multiplied by the average energy of the BXR photons produced
by the BXR converter as shown in Figure 1. The results of the calculation of the average energy of BXR
photons emitted forward and its relation to the thickness of the converter material are shown in Figure
3. So, the average energy of BXR photons emitted forward in the graph in Figure 3 is the result of the
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The 11th National Physics Seminar (SNF 2022) IOP Publishing
Journal of Physics: Conference Series 2377 (2022) 012048 doi:10.1088/1742-6596/2377/1/012048
product of the average energy of the BXR photons produced by the BXR converter in the graph in Figure
1 and the fraction value of the x-ray photon beam emitted forward in the graph in Figure 2.
In general, the value of the graph in Figure 1 for the three BXR converter materials has an upward
trend (at first it rose significantly and then stabilized), while the value of the graph in Figure 2 continues
to fall so that when the two graphs the values are multiplied, it will produce a graph in Figure 3 where
the trend initially increases until maximum value, then decreases. So, from the graph in Figure 3, it can
be obtained that the optimum thickness of the BXR converter material is capable of producing maximum
BXR photon energy scattered forward from the electron kinetic energy of 10 MeV. The BXR converter
material made of tantalum, tungsten, lead has an optimum thickness of 2.0 mm, 1.8 mm, 2.8 mm and
can convert 10 MeV electron kinetic energy into maximum BXR photon energy scattered forward of
2.1137 MeV, 2.1287 MeV, 2.1850 MeV. This means that the optimum thickness of the BXR converter
material is inversely proportional to the density of the converter material. The greater the density value
of the converter material, the smaller the value of the optimum thickness of the converter material.
Meanwhile, the maximum BXR photon energy value is directly proportional to the atomic number of
the converter material. The greater the atomic number of the converter material, the greater the
maximum BXR photon energy produced.
3.0 26
Forward Scattered BXR Conversion Efficiency (%)
Forward Scattered BXR Energy (MeV)
24
2.5
22
2.0
20
1.5 18
Ta
16
1.0 Ta
W
14 W
0.5 Pb
12 Pb
0.0 10
0.0 1.0 2.0 3.0 4.0 5.0 6.0 7.0 8.0 0.0 1.0 2.0 3.0 4.0 5.0 6.0 7.0 8.0
X-Ray Converter Thickness (mm) X-Ray Converter Thickness (mm)
Figure 3. The relationship of the forward scattered Figure 4. The relationship of the forward scattered
BXR average energy to the converter thickness. BXR conversion efficiency to the converter
thickness.
Figure 3 provides information on the optimum thickness of the BXR converter material and the
maximum BXR photon energy scattered forward, but it does not provide information on what percentage
(%) of the maximum efficiency of the converter material is able to convert the kinetic energy of 10 MeV
electrons into the energy of BXR photons scattered forward. Therefore, the maximum efficiency of the
BXR converter material is important to calculate and know, namely the maximum BXR photon energy
scattered forward divided by the electron kinetic energy of 10 MeV and expressed in percent (%).
The graph in Figure 4 shows the relation of the forward-scattered BXR conversion efficiency to the
thickness of the converter material. Because the conversion efficiency of the x-ray converter is
calculated using the electron kinetic energy of 10 MeV as the divider, the graphic pattern in Figure 4 is
similar to the graphic pattern in Figure 3. From the graph in Figure 4, it can be obtained information
about the maximum conversion efficiency of BXR scattered forward for tantalum, tungsten, lead,
21.137%, 21.287%, 21.850%, respectively, with the optimum thickness of each converter material is
2.0 mm, 1.8 mm, 2.8 mm, respectively.
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The 11th National Physics Seminar (SNF 2022) IOP Publishing
Journal of Physics: Conference Series 2377 (2022) 012048 doi:10.1088/1742-6596/2377/1/012048
The optimum thickness and maximum conversion efficiency of the tantalum-based BXR converter
in this study when compared with the results of DePriest’s study [15] are shown in Table 1. The optimum
thickness of the tantalum converter in this study was 2.00 mm, while the result of DePriest’s study was
2.268 mm. So the optimum thickness of tantalum as a result of this study is 11.82% smaller than the
result of DePriest’s study. Then the maximum conversion efficiency of the tantalum converter in this
study was 21.1%, while the result of DePriest’s study was 16.5%. So the maximum conversion
efficiency of the result of this study is 28.12% greater than the result of DePriest’s study.
Table 2 compares this study’s results with the results of other studies regarding the optimum
thickness and maximum conversion efficiency of the tungsten-based BXR converters. The optimum
thickness of the Tungsten converter in this study was1.80 mm. The result of this study is greater than
the results of other studies, namely Tsechanski et al by 1.64 mm (9.76% larger) [16], Berger et al by
1.36 mm (32.35% larger) [17], Alhagaish and Sakharov by 1.61 mm (11.80% larger) [4]. Then the
maximum conversion efficiency of the Tungsten converter in this study was 21.3%, which means it is
smaller than the results of Tsechanski et al’s study by 23.1% (7.79% smaller) [16], Alhagaish and
Sakharov by 23.2 % (8.19% smaller) [4], but greater than the result of the study of Berger et al, namely
19.0% (12.11% larger) [17].
4. Conclusion
Based on the description of the results and discussion above, it can be concluded that the MCNPX code
simulation has succeeded in determining the optimum thickness of the BXR converter material. The
BXR converter material made of tantalum, tungsten, and lead has an optimum thickness of 2.0 mm, 1.8
mm, and 2.8 mm, respectively. Each is capable of converting 10 MeV electron kinetic energy into
maximum forward scattered BXR photon energy of 2.1137 MeV, 2.1287 MeV, and 2.1850 MeV,
respectively. The maximum conversion efficiency for tantalum, tungsten, and lead converter materials
are 21.137%, 21.287%, and 21.850%, respectively. The optimum thickness value of the BXR converter
material is inversely proportional to the density of the converter material. At the same time, the value of
the maximum BXR photon energy and maximum BXR conversion efficiency scattered forward by the
converter material is directly proportional to the atomic number of the x-ray converter material. These
results can be used as a reference in the design of the BXR converter for the 10 MeV high-energy
electron accelerator.
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The 11th National Physics Seminar (SNF 2022) IOP Publishing
Journal of Physics: Conference Series 2377 (2022) 012048 doi:10.1088/1742-6596/2377/1/012048
5. Acknowledgment
This research is supported by the Research Organization for Nuclear Energy, National Research and
Innovation Agency of Indonesia under the Innovative Electron Accelerator Project.
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